Leo Compatibility Most Least Compatible Signs MyPanditLibra passion most suitable zodiac signs are gemini, water bearer, and ram. When it comes to matters of the love, Libra seeks harmony and understanding above all else. Gemini can offer adventure and fun to the bond, while The Water Bearer shares Libra's appreciation for wisdom and innovation. Aries, known for their passion, can ignite a flame in Libra's soul. Libra and these signs create a balanced and rewarding union.